Abstract
The theory of the Brillouin scattering from the surface of a semi-infinite medium, developed previously, is extended to coated surfaces of cubic materials. The Brillouin cross section is obtained for any scattering geometry and for p and s polarisation of the incident and scattered light. The formulae for the cross section contain contributions from the ripple and the elasto-optic scattering mechanisms for the film as well as for the substrate. The theory is applied to a silica film deposited on crystalline silicon and the behaviour of the cross section against the film thickness is investigated. The authors find that there are strong interference effects among the various contributions to the cross-section, so that the intensity of the spectral lines dramatically oscillates by changing the thickness. Although in general the ripple scattering mechanism is the dominant one it is found that the elasto-optic coupling in the silica film is not negligible and sometimes is even prevailing. The discrete phonon spectrum (Rayleigh, Sezawa, Lamb modes) and the continuous spectrum (resonances, mixed modes) are both studied.
Published Version
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