Abstract

The results of the calculation on magnetization (M) for diluted magnetic semiconductor Pb1-xEuxSe are reported. Our calculation includes two distinct contributions namely contribution from the localized magnetic impurity (Mi) and contribution from the band effect (Mb). Mi has been calculated using a three-spin cluster model which comprises the clusters consisting of one-spin (M1), two-spins (M2) and three-spins (M3). Moreover, M3 includes both open triplets (Mot) and closed triplets (Mct). The statistical distribution of the different clusters has been considered using random distribution approximation in the dilute limit. The contributions from these clusters to the magnetization have been evaluated using a modified Heisenberg's exchange Hamiltonian in the nearest approximation. The magnetization has been calculated as a function of magnetic field and impurity concentration. The band effect includes the contribution from lattice diamagnetism(χlatt). This mechanism has been considered in the effective mass formalism using a two-band k→.π→model. Our calculated values of M compare very well with experimental data where available.

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