Abstract

Present paper investigate theoretically dielectric properties such as dielectric constant, soft mode frequency and tangent loss by considering two sub lattice pseudospin, spin-lattice coupled mode model (PLCM) and adding third and fourth-order anharmonic (phonon) and spin-lattice interaction terms and using thermal Green’s function (double time) method expression for dielectric constant, soft mode frequency, and tangent loss is derived for TGS crystal. Model value have been fitted in expression and their temperature dependence have been calculated for TGS crystal. Theoretical results have been correlated with experimental results of (Aravzhi et al 1997), which is approximate close to experimental results.

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