Abstract

Picosecond laser ellipsometry has been used in the visible to estimate for the first time the index of refraction of highly oriented pyrolitic graphite samples at high temperatures. While recent experiments seem to indicate that molten graphite behaves in many respects as a metal, investigation of optical properties with picosecond laser pulses consistently shows a reduced reflectivity value as soon as the threshold value of laser fluence for surface melting is exceeded. This occurrence may be interpreted as a reduced conductivity of the liquid phase. The experimental conditions are discussed, and in particular, the possible occurrence of optically thick layers of matter in front of the hot surface during the measurements is evaluated.

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