Abstract

A new method for ionic transfer detection is called Doppler Broadening S parameter of Positron Annihilation Spectroscopy (PAS) is used to study polysiloxane electrolytes with ethylene oxide (EO) side chains and carbonate electrolytes. First, the polymer electrolytes are modified to enhance contact with an acrylate, and an increase in the lengths of the EO chains is shown to decrease the resistance of the transition interface layer at the pristine electrode surface. Second, an ionic transfer study of the electrode surface after electrochemical reactions showed that the polymer electrolytes have a greater effect on the interface transition layers than did the carbonate electrolytes. In addition, a continuity phase including a chemical membrane that is formed from carbonate electrolytes during electrochemical reactions and the enhancing ionic transfer benefits is found by this new detecting methodology.

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