The influence of laser-induced alignment on Z-scan properties of 2D carbon nanomaterials suspension dependent on polarization

Abstract

The Z-scan technique uses a single beam that can be used for observing the nonlinear or optical limiting properties of materials. For the first time, the Z-scan properties dependent on the polarization of 2D carbon nanomaterial suspension were experimentally investigated using optical Z-scan technology. The Z-scan curves of graphene and graphene oxide (GO) in N-methyl-2-pyrrolidinone suspensions exhibited strong polarization-dependent characteristics. In paper, a reverse saturated absorption (RSA) dip surrounded the lens focus when the horizontal polarized beam was focused in the suspension, and two saturated absorption (SA) peaks appeared adjacent to the dip. However, for the vertical polarized beam, only one RSA dip surrounded the lens focus, and the threshold was higher than the SA for a horizontally polarized beam. The transmission of RSA for the GO suspension was evidently lower than that of the graphene suspension. The polarization-dependent characteristic can be ascribed to the laser-induced alignment in case the suspension is moved in or out of the beam focal point. Furthermore, the polarization-dependent 2D carbon nanomaterial suspension can be applied in several practical purposes such as 2D material-based optical and opto-fludic devices.