Abstract
Revealing the evolution of nanoscale third bodies confined between sliding surfaces is essential to understanding the friction and electrical properties for solid contacts. Here, with graphite/graphite contacts in structural superlubricity, a state of no wear and ultralow friction, we in situ reveal the morphological evolution of a third body layer introduced by air through measuring friction and conductance during cyclic hold-slide tests. The directional transport of confined molecules causes apparent elastic deformation of the third body layer, leading to local graphite/graphite direct contact. Together with a proposed quantum tunneling effective thickness (deff) model, a constant volume of third bodies with a sub-nm thickness is observed. Our work provides a feasible approach to investigate the kinetics of substances under nanoscale confinement.
Published Version
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