Abstract
The He(I) and He(II) photoelectron spectra of a series of Fe 2(CO) 6LL 1-type complexes (L = L 1 = S, ( i-propyl)S; L,L 1 = t-but of an all-electron, ab initio SCF MO calculation on Fe 2(CO) 6S 2 and of extended CNDO calculations on related molecules. Assignments given ar He(I)/He(II) intensity differences, and on comparison with related molecules. The coordination of the bridging ligands to the metal centres and the nature of the metal—metal interactions are discussed.
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