Abstract
The effect of altering the excitation rate on the emission energy of a photonic band edge liquid crystal laser has been investigated. The results showed that for excitation energies greater than 18 µJ/pulse, an increase in the excitation rate from 1 to 20 Hz caused a reduction in the total emission energy of the photonic band edge liquid crystal laser of up to 90%. In order to establish the cause of this reduction several factors were considered: dye bleaching, thermal/density effects and director-axis reorientation (either by virtue of a light-induced torque or other effects such as a flow-induced orientational decay). Although some dye bleaching was observed, the main factor responsible for the reduction in the overall emission efficiency was found to be nonlinear changes in the director-axis reorientation. Furthermore, our results suggest that the director-axis reorientation is the result of an optical torque, enhanced by the presence of the dye, which for a chiral nematic liquid crystal results in a dilation of the helical pitch.
Published Version
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