Abstract
The effect of third nearest neighbor interactions on the thermodynamic functions of interstitial solid solutions has been investigated. The free energy of the solution crystal was obtained by the cumulant expansion technique. It has been shown that even strong third nearest-neighbor interactions have a negligible effect on the partial configurational entropy of the solute atoms. The effect of these interactions on the partial enthalpy is much larger, but the general form of the variation of the partial enthalpy with temperature and composition round previously in simpler statistical mechanical models is conserved.
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