Abstract
The interaction of fluoride ion with manganese(II) ion is studied in aqueous and nonaqueous systems. The electron paramagnetic resonance spectra show that in water and mixed solvents, a fluoride complex forms with manganese that is apparently a dimer similar to the μ-oxo-bridged species formed commonly by iron(III) with similar changes in the magnetic properties. However, a novel hexafluoromanganate(II) complex may be made inside zeolite cages which displays a characteristic 42-line EPR spectrum with line widths of 6.7 G which correspond to electron relaxation times of 9.8 ns
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