Abstract
The use of Sm{sub 2}O{sub 3} as a catalyst for the oxidative coupling of methane has been well studied and documented. However, detailed information on the surface of a working Sm{sub 2}O{sub 3} catalyst and the overall carbon reaction pathway is unknown. This communication presents results that delineate completely for the first time the nature of the surface-reaction steps of Sm{sub 2}O{sub 3} and quantifies the working surface under steady-state reaction conditions.
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