Abstract

The fluidized reactor is widely used in a number of chemical processes due to its high gas-particle contacting efficiency and excellent performance on solid mixing. An improved numerical framework based on the multiphase particle-in-cell (MP-PIC) method has been developed to simulate the processes of gas–solid flow and chemical reactions in a fluidized bed. Experiments have been carried out with a 3-MW circulating fluidized bed with a height of 24.5 m and a cross section of 1 m2. In order to obtain the relationship between pollutant discharge and operating conditions and to better guide the operation of the power plant, a series of tests and simulations were carried out. The distributions of temperature and gas concentration along the furnace from simulations achieved good accuracy compared with experimental data, indicating that this numerical framework is suitable for solving complex gas–solid flow and reactions in fluidized bed reactors. Through a series of experiments, the factors affecting the concentration of NOx and SOx emissions during the steady-state combustion of the normal temperature of powder coke were obtained, which provided some future guidance for the operation of a power plant burning the same kind of fuel.

Highlights

  • The fluidized reactor is widely used in a number of chemical processes due to its high gas-particle contacting efficiency, wide fuel adaptability, and excellent performance on solid mixing

  • For the sake of verifying the accuracy of the 3D computational fluid dynamics (CFD) model based based on the multiphase particle-in-cell (MP-PIC) method, a set of stable operating conditions were selected for simulation

  • As a new type of fluidized bed fuel, powder coke, which is carbonized by coal, has been studied in this paper for its fluidized combustion and pollutant emission characteristics

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Summary

Introduction

The fluidized reactor is widely used in a number of chemical processes (e.g., circulating fluidized bed boiler combustion, biomass pyrolysis, catalytic reaction, and conceptual fluidized bed nuclear reactor [1,2,3,4]) due to its high gas-particle contacting efficiency, wide fuel adaptability, and excellent performance on solid mixing. Its structure is blocky and its color is light black. It is a fuel and reducing agent for ferroalloys, fertilizers, calcium carbide, blast furnace injection, and other applications. As a new type of fluidized bed boiler fuel, it has a relatively high fixed carbon content; low ash, aluminum, and sulfur contents; and its specific resistance and chemical activity are high. Vigorous development of circulating fluidized bed (CFB) boiler combustion technology for special fuels has important strategic significance for broadening the future circulating fluidized bed market

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