Abstract
The reactions between silver and sulfur clusters are studied with a laser double ablation reactor. The main reaction products are [AgS4]+, [AgS8]+, [AgS12]+, and [AgS16]+, which have different compositions from those of Ag/S clusters produced from Ag/S mixed sample by laser ablation. The photolysis of the products with a 193 nm excimer laser indicates that [AgS12]+ and [AgS16]+ have a photodissociation efficiency much higher than that of [AgS4]+ and [AgS8]+. The structure of the products and the mechanism of the reactions to form products [AgS12]+ and [AgS16]+ are discussed.
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