Studies on catalytic epoxidation reaction cycle with titanium silicalite-1 (ts-1) cluster model: Ts-1 peroxide formation and epoxidation reaction

Hiroaki Munakata,Yasunori Oumi,Akira Miyamoto

doi:10.1016/s0167-2991(99)80071-8

Studies on catalytic epoxidation reaction cycle with titanium silicalite-1 (ts-1) cluster model: Ts-1 peroxide formation and epoxidation reaction

Hiroaki Munakata, Yasunori Oumi + Show 1 more

https://doi.org/10.1016/s0167-2991(99)80071-8

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Journal: Studies in Surface Science and Catalysis	Publication Date: Jan 1, 1999
Citations: 3

Affiliation: Tohoku University

#Titanium Silicalite-1 #Activation Of Hydrogen Peroxide + Show 8 more

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Abstract

Abstract DFT calculations on TS-1 model clusters showed that activation of hydrogen peroxide on titanium silicalite-1 (TS-1) led to form a water adduct of peroxy TS-1 complex, which was examined as an oxidizing agent in the catalytic reaction cycle to produce epoxyethane from ethene.

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