Abstract
We have recently measured the surface phonon spectrum of the ordered binary alloy Cu 3Au(001). In addition to the Rayleigh wave, we observe a higher energy mode which may be interpreted as the “folded” Rayleigh mode or “optical” surface mode. Using a harmonic pair potentials fit to the inelastic neutron scattering data of Katano et al, 13 we find that the force constant between the first and second layer Cu atoms must be stiffened by 20% with respect to the bulk value in order to match the “folded” Rayleigh mode.
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More From: Journal of Electron Spectroscopy and Related Phenomena
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