Abstract
This study examines the impact of mechanical vibration on the carbonation process of steel slag, a substantial byproduct of steel production. Employing a methodical experimental design that modulates mechanical vibration frequencies, the research reveals that mechanical vibration markedly influences carbonation, with an optimal frequency of 180 Hz leading to a 27.5 % increase in compressive strength of steel slag compact and an increase in CO2 uptake of 6.8 %. The application of vibration appears to catalyze the conversion of calcium-rich minerals into well-formed rhombohedral calcite, which emerges as the predominant carbonation product. Mechanism analysis suggests that vibration-induced particle redistribution creates new reaction surfaces, thereby accelerating the carbonation process. However, the effect is more pronounced in early stages, with diminishing returns as carbonation progresses. These pivotal findings propose an innovative strategy to augment the efficiency of carbonation and the inherent material properties of steel slag, thereby fostering a more sustainable approach to the utilization of industrial byproducts.
Published Version
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