Abstract

Reduced emissions of nitrogen (N) in Europe have resulted in decreasing atmospheric deposition since 1990. Long-term data (1988–2017) from four small Norwegian catchments located along gradients in N deposition, rainfall, and organic carbon (C) show different responses to 25–30% reductions in N deposition during the same period. At three sites the decreased N deposition caused reduced leaching of nitrate to surface water, whereas the westernmost site showed no decrease, probably due to thin soils with low C:N ratio, poor vegetation cover and high precipitation. The loss of total N to streamwater constituted 30–50% of the N deposition. Losses via denitrification are unknown but assumed to be low, as a major fraction of the catchments are well-drained. Hence, the study sites seem to continue to accumulate N, presumably mostly in soil organic matter. Although atmospheric N deposition has declined, ambient loads might still exceed long-term sustainable levels in these vulnerable ecosystems.

Highlights

  • Emissions of sulphur oxides (SOx), nitrogen oxides (NOx) and reduced nitrogen (NHx) in Europe have been reduced by approximately 90, 55 and 20%, respectively, since 1990 (EEA 2017)

  • Reduced deposition of sulphate (SO4) and sea-salts has resulted in an increase in dissolved organic carbon (DOC) in surface waters (Monteith et al 2007), a proxy for dissolved organic matter (DOM) which is a vector for transport of organic N

  • Concentrations of non-marine SO4 are highest at Birkenes (1.3 mg L-1) and somewhat lower in the other three catchments (0.6-0.7 mg L-1)

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Summary

Introduction

Emissions of sulphur oxides (SOx), nitrogen oxides (NOx) and reduced nitrogen (NHx) in Europe have been reduced by approximately 90, 55 and 20%, respectively, since 1990 (EEA 2017). In Fennoscandia there were reports of increasing N concentrations in upland surface waters during the 1980s and 1990s (Agren 1983; Lepisto 1995; Kaste et al 1997). Many of these ecosystems are sensitive to acidification. They have thin soils and sparse vegetation and a limited capacity to retain N from atmospheric deposition

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