Abstract
Abstract Most research of stratospheric aerosol injection (SAI) for solar radiation modification (SRM) has focused on injection of \ce{SO2}. However, the resulting sulfuric acid aerosols lead to considerable absorption of terrestrial infrared radiation, resulting in stratospheric warming and reduced cooling efficiency. Recent research suggests that solid particles, such as alumina, calcite or diamond, could minimize these side effects. Here we use, for the first time, the atmosphere-ocean-aerosol-chemistry-climate model SOCOLv4.0, incorporating a solid particle scheme, to assess the climatic impacts of SAI by these injection materials. For each substance, we model tropical SAI by means of constant yearly injection of solid particles, aimed to offset the warming induced by a high-GHG emission scenario over the 2020-2100 period by 1 K. We show that solid particles are more effective than sulfur at minimising stratospheric heating, and the resulting side-effects on the general atmospheric circulation, stratospheric moistening, and tropopause height change. As a result, solid particles also induce less residual warming over the Arctic, resulting in greater reduction of GHG-induced polar Amplification compared to sulfuric acid aerosols. Among the materials studied here, diamond is most efficient in reducing global warming per unit injection, while also minimizing side effects.
Published Version
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
