Abstract
The Atmospheric Chemistry Experiment (ACE) Fourier transform spectrometer (FTS) has been measuring water vapor and methane in the stratosphere and mesosphere from low Earth orbit since 2004. Recently, substantial increases in water vapor in the upper atmosphere were observed with the MLS and SABER satellite instruments. The main source of water vapor in the upper atmosphere is methane oxidation. ACE-FTS data show substantial water and methane increases, and confirm that the methane increases are too small to explain the water increases. Therefore, changes in the transport of water across the tropical tropopause layer and in atmospheric dynamics are responsible for the positive water trends.
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More From: Journal of Quantitative Spectroscopy and Radiative Transfer
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