Stability of a layered reactive channel flow

Abstract

We analyse the linear stability of a reactive plane Poiseuille flow, where a reactant fluid A overlies another reactant B in a layered fashion within a two-dimensional channel. Both reactants are miscible and have the same viscosity, while upon reaction, they produce either a less or more-viscous product fluid C . The reaction kinetics is of simple A + B → C type, and the production of C occurs across the initial contact line of reactants A and B in a mixed zone of small and finite width. All three fluids have the same density. We demonstrate the effects of various controlling parameters such as the log-mobility ratio, Damköhler number, Schmidt number, Reynolds number, position and thicknesses of the reactive zone on the stability characteristics. We show that a tiny viscosity stratification by the reaction destabilizes the flow at a moderate (10–1000) and even at low Reynolds numbers (0.01–1). The maximum growth occurs for shorter waves than for the Tollmien–Schlichting eigenmode, and the ranges of unstable wavenumbers are wider than that known for non-reactive channel flow systems. In most cases, the instability occurs due to the overlap of the critical layer with the viscosity-stratified layer. Surprisingly for some parameters, it is observed that the reaction can make σ M decrease with increasing Reynolds number.