Abstract

Low-temperature magnetic ac susceptibility measurements of single-crystal dipolar spin ice Dy${}_{2}$Ti${}_{2}$O${}_{7}$ are presented. The relaxation is found to exhibit thermally activated Arrhenius behavior with an activation energy of 9.79 K ($\ensuremath{\sim}$$9{J}_{\mathrm{eff}}$), which is not consistent with a simple scaling of $6{J}_{\mathrm{eff}}$, as previously found for Ho${}_{2}$Ti${}_{2}$O${}_{7}$. There are distinct quantifiable differences between Dy${}_{2}$Ti${}_{2}$O${}_{7}$ and Ho${}_{2}$Ti${}_{2}$O${}_{7}$ absorption spectra. The measured dynamics does not agree with simulations based on current magnetic monopole theory nor thermal relaxation measurements, but instead freezes out at a faster rate.

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