Abstract

Spatiotemporal information about light pulse propagation obtained with femtosecond temporal resolution plays an important role in understanding transient phenomena and light–matter interactions. Although ultrafast optical imaging techniques have been developed, it is still difficult to capture light pulse propagation spatiotemporally. Furthermore, imaging through a three-dimensional (3-D) scattering medium is a longstanding challenge due to the optical scattering caused by the interaction between light pulse and a 3-D scattering medium. Here, we propose a technique for ultrafast optical imaging of light pulses propagating inside a 3D scattering medium. We record an image of the light pulse propagation using the ultrashort light pulse even when the interaction between light pulse and a 3-D scattering medium causes the optical scattering. We demonstrated our proposed technique by recording converging, refracted, and diffracted propagating light for 59 ps with femtosecond temporal resolution.

Highlights

  • Spatiotemporal information about light pulse propagation obtained with femtosecond temporal resolution plays an important role in understanding transient phenomena and light–matter interactions

  • Digital light-in-flight recording by holography (DLIF holography)[24,25,26,27,28] was developed for observing light pulse propagation

  • Even though the technique, which allows the observation of light pulse propagation as a motion picture with a single-shot, has been shown to perform well, observing light pulse propagation in a 3-D scattering medium by DLIF holography has not been reported yet

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Summary

Introduction

Spatiotemporal information about light pulse propagation obtained with femtosecond temporal resolution plays an important role in understanding transient phenomena and light–matter interactions. We propose a technique for ultrafast optical imaging of light pulses propagating inside a 3D scattering medium. Capturing the light pulse propagation inside a three-dimensional (3-D) scattering medium, which is closely related to the optical scattering properties, is desirable for establishing techniques for focusing light in deep tissue for high-resolution imaging and precision laser ­therapy[6,7,8]. LIF holography can provide a motion picture of light pulse propagation inside a 3-D scattering ­medium[21]. Digital light-in-flight recording by holography (DLIF holography)[24,25,26,27,28] was developed for observing light pulse propagation. We present the observation of light pulse propagation inside a 3-D scattering medium by DLIF holography. The results presented here are a significant step forward in revealing ultrafast phenomena related to light pulse propagation inside 3-D scattering media

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