Abstract

The Qiandao Lake Basin (QLB), which occupies low hilly terrain in the monsoon region of southeastern China, is facing serious environmental challenges due to human activities and climate change. Here, we investigated source attribution, transport processes, and the spatiotemporal dynamics of nitrogen (N) movement in the QLB using the Soil and Water Assessment Tool (SWAT), a physical-based model. The goal was to generate key localized vegetative parameters and agronomic variables to serve as credible information on N sources and as a reference for basin management. The simulation indicated that the basin’s annual average total nitrogen (TN) load between 2007 and 2016 was 11,474 tons. Steep slopes with low vegetation coverage significantly influenced the spatiotemporal distribution of N and its transport process. Monthly average TN loads peaked in June due to intensive fertilization of tea plantations and other agricultural areas and then dropped rapidly in July. Subsurface flow is the key transport pathway, with approximately 70% of N loads originating within Anhui Province, which occupies just 58% of the basin area. The TN yields of sub-basins vary considerably and have strong spatial effects on incremental loads entering the basin’ major stream, the Xin’anjiang River. The largest contributor to N loads was domestic sewage (21.8%), followed by livestock production (20.8%), cropland (18.6%), tea land (15.5%), forest land (10.9%), atmospheric deposition (5.6%), orchards (4.6%), industry (1.4%), and other land (0.8%). Our simulation underscores the urgency of increasing the efficiency of the wastewater treatment, conserving slope land, and optimizing agricultural management as components of a comprehensive policy to control N pollution in the basin.

Highlights

  • The nitrogen (N) cycle is dynamic and strongly influenced by both human activities and physical conditions, especially in environmentally sensitive areas that are prone to nutrient pollution [1,2].Agricultural practices and domestic sewage account for a substantial proportion of released N, which subsequently enters waterways via pathways that are diverse and poorly understood

  • Appropriate calibration with parameters that are optimized for the Qiandao Lake Basin (QLB) is important, especially for tea, which is intensively managed, known to have undergone considerable expansion during the study period, and recognized to be an important source of nutrient pollution [42,43]

  • We found that sub-basin to sub-basin heterogeneity in total nitrogen (TN) loads and yields was pronounced across the QLB, where four clustered sub-basins located upstream in Anhui Province stand out as a hotspot, because of their extensive and intensive contributions to TN pollution

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Summary

Introduction

The nitrogen (N) cycle is dynamic and strongly influenced by both human activities and physical conditions, especially in environmentally sensitive areas that are prone to nutrient pollution [1,2].Agricultural practices and domestic sewage account for a substantial proportion of released N, which subsequently enters waterways via pathways that are diverse and poorly understood. Water 2020, 12, 1075 features and geomorphological factors, including intense rainfall, steep slopes, and the presence of erodible soils, exacerbate N emission, transport, and export, adding complexity to the problem of pollution control [1,2,3]. Against this backdrop, access to comprehensive information about spatiotemporal patterns of N distribution becomes a primary concern for pollution management. Physical-based models are powerful tools to provide detailed information about the key driving factors of N release and transport.

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