Spatiotemporal distribution and potential sources of atmospheric microplastic deposition in a semiarid urban environment of Northwest China.

Abstract

In this study, the spatiotemporal distribution of microplastic deposition was investigated through ordinary Kriging interpolation, and the potential sources of microplastic deposition were identified by using Hybrid Single-Particle Lagrangian Integrated Trajectory model. The results showed that the total deposition flux of microplastics ranged from 79.5 to 810.0 p/(m2·d). The shapes of microplastics could be divided into 4 shapes: fiber, fragment, film, and pellet. Seven polymer types of microplastics were identified, including polyamide (PA), polyethylene (PE), polyethylene terephthalate (PET), polymethyl methacrylate (PMMA), polypropylene (PP), polystyrene (PS), and polyvinyl chloride (PVC). Most microplastics were tiny and small sizes (≤ 500 μm) and colorless. Through model analysis and survey, microplastic deposition came from the study region, and the potential sources might be plastic products and wastes. The seasons with the highest and lowest total deposition flux were summer (535.5 p/(m2·d)) and winter (197.5 p/(m2·d)), respectively. The months of the highest and lowest total deposition flux were June 2021 (681.4 p/(m2·d)) and January 2022 (112.2 p/(m2·d)), respectively. Most fibers (PET, PA, PP) and fragments (PP) were distributed in populous areas such as commercial centers and residential areas. Abundant fragments (PET, PS, PE) and films (PE, PVC) were distributed around salvage stations. Almost all of the pellets (PE, PMMA) were found in the factory. Our results suggested that the temporal distribution of microplastic deposition was influenced by precipitation and mean temperature of air, and the spatial distribution of microplastic deposition was influenced by sources and population density.