Solid state dye lasers with scattering feedback

Abstract

Over the last decade, significant advances have been made toward the development of practical, tunable solid state dye lasers, which resulted in improved lasing efficiency with reduced dye photodegradation. To achieve this goal, a “chemical” approach was followed, where attention was focused onto the particular dye/host interaction and compatibility, specifically choosing already existing hosts for a given dye, synthesizing new dyes and/or matrices, or chemically modifying existing ones. Nevertheless, this approach was limited by a single fact learnt from the experience: there is no universal matrix which optimizes the efficiency and photostability of all dyes. This limitation could be overcome by following a “physical” approach, where the emission properties of the active medium are tailored by means of physical and structural modifications of the dye host.Following this approach, in this paper recent theoretical and experimental work is reviewed where it is demonstrated that following a simultaneous “physical” and “chemical” approach to tailor the emission properties of the host materials for solid state dye lasers, may lead, under specific circumstances, to the improvement of both the laser efficiency and photostability. In particular, it is demonstrated that optical scattering is not always detrimental either to conventional bulk lasers (laser rods or colloidal suspensions) or to integrated devices, but may give place, on the contrary, to dramatic improvements in the laser operation of organic (hybrid) laser rods, and to alternative ways of obtaining laser light from integrated devices based on the phenomenon of coherent random lasing, where feedback is provided by light scattering in an appropriate medium, without the need to manufacture complex periodic structures in the substrate. The processing and pumping flexibility of these materials, together with their low cost and capability of efficient emission across the whole visible spectrum makes them very attractive for the fabrication and development of coherent light sources suitable for integration in optoelectronic and disposable spectroscopic and sensing devices.