Abstract

The principal elements of the 13 C NMR chemical shift tensors have been determined for three square-planar tetracyanometalates, K 2 Ni(CN) 4 .H 2 O, K 2 Pd(CN) 4 -3H 2 O, and K 2 Pt(CN) 4 .3H 2 O, from the solid-state 13 C NMR powder patterns. The orientation of the 13 C chemical shift tensor is partially assigned on the basis of the dipolar coupling analysis to 14 N

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