Abstract

Yield-stress materials such as structurally complex formulations of paints, slurries, and waxes have been long ubiquitous in the coating industry, though the practice of coating engineering remains largely empirical as the fundamental role of viscoplasticity due to the yield stress of the coating material in most coating applications is still unclear. Here, we couple a recent harmonic mean viscosity regularization for the Bingham model with a well-established finite element/elliptic mesh generation method for free surface flows to present a detailed computational study of slot coating applications of viscoplastic materials. By neglecting inertia and focusing on the downstream section of a slot coater, we introduce suitable dimensionless parameters to discuss a comprehensive set of results that unravels a striking impact of viscoplasticity on the flow dynamics and low-flow limit. We show that viscoplastic effects have major implications to the velocity field and recirculation pattern in the coating bead as well as to the development length and free surface in the film formation region. Most importantly, we find that viscoplastic effects markedly widen the operating window of the process, delaying the onset of the low-flow limit and thereby suggesting that structurally complex yield-stress materials may be used to coat thinner films and/or at higher speeds than predicted by the standards far established for simple Newtonian liquids.

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