Abstract

Formation of nanodomain structures during cooling after pulse heating by infrared laser has been studied in congruent lithium tantalate (CLT) and lithium niobate (CLN) single crystals. In situ study of the domain structure evolution allowed to reveal that in CLN the isolated domains appeared at the edges of the irradiated zone and grew to the center. In contrast, the quasi-regular stripe domain structure appeared in CLT near the edge of irradiated zone. The difference has been attributed to lower Curie temperature and larger pyroelectric coefficient of CLT. The self-organized domain structures can be used for periodical poling with submicron periods.

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