Abstract
In order to understand how the doping with self-assembled nanorods of different sizes and concentrations as well as applied magnetic fields affect the critical current anisotropy in YBa2Cu3O7−x (YBCO) thin films close to YBCO c-axis, we present an extensive and systematic computational study done by molecular dynamics simulation. The simulations are also used to understand experimentally measured Jc(θ) curves for BaHfO3, BaZrO3 and BaSnO3 doped YBCO thin films with the help of nanorod parameters obtained from transmission electron microscopy measurements. Our simulations reveal that the relation between applied and matching field plays a crucial role in the formation of Jc(θ)-peak around YBCO c-axis (c-peak) due to vortex-vortex interactions. We also find how different concentrations of different size nanorods effect the shape of the c-peak and explain how different features, such as double c-peak structures, arise. In addition to this, we have quantitatively explained that, even in an ideal superconductor, the overdoping of nanorods results in decrease of the critical current. Our results can be widely used to understand and predict the critical current anisotropy of YBCO thin films to improve and develop new pinscapes for various transport applications.
Highlights
In order to understand how the doping with self-assembled nanorods of different sizes and concentrations as well as applied magnetic fields affect the critical current anisotropy in YBa2Cu3O7−x (YBCO) thin films close to YBCO c-axis, we present an extensive and systematic computational study done by molecular dynamics simulation
One of the most common features of nanorods experimentally encountered in thin films is their splay and fragmentation, the effects of which to YBCO c-axis peak have already been comprehensively studied in[24], where the increasing splay of nanorods was reported to decrease the absolute value of critical current
We have extensively investigated the effects of the applied magnetic field, nanorod size and their concentration on the critical current isotropy and explained them via the dynamics of the vortices
Summary
In order to understand how the doping with self-assembled nanorods of different sizes and concentrations as well as applied magnetic fields affect the critical current anisotropy in YBa2Cu3O7−x (YBCO) thin films close to YBCO c-axis, we present an extensive and systematic computational study done by molecular dynamics simulation. The intrinsic anisotropy of the critical current, in thin films and coated conductors, can be modified by adding impurities within the lattice of YBCO which pin the vortices restricting their movement. A topic of interest has been to add both point-like nanodots and nanorods within the YBCO lattice simultaneously This has been achieved by doping YBCO simultaneously with both BYTO and BYNO (referred as BYNTO) with an additional rare earth oxide, leading to continuous niobiate/tantalate nanorods and rare-earth oxide nanoparticles[19]. A huge topic of interest has been how different dopants affect the isotropy of angular dependent critical current Jc(θ)
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