Abstract

The activity size distributions of cosmogenic 7Be and the longer living radon progenies 210Pb and 210Po in urban aerosols were measured for summers and winters from, 2014 to the end of 2017. The average seasonal activity median aerosol diameters (AMADs) and mass median aerosol diameters (MMADs) calculated for summer ranged from 0.329 μm to 0.733 μm and were ordered AMADBe-7, <AMADPb-210,<AMADPo-210,<MMAD, whereas for winter, these values were from 0.420 μm to 0.538 μm but were differently ordered:AMADPo-210,<AMADBe-7,<AMADPb-210,<MMAD. The prevailing occurrence of 210Po in particles of the smallest diameter during winter can be explained by the remarkable additional anthropogenic emission of this radionuclide from coal combustion. This was confirmed with principal component analysis (PCA) of the AMAD data.

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