Abstract

Neutron-energy-gain spectra have been measured in (NH4)2CO3, (NH4)2HC6H5O7, and NH4C2H3O2 at 20°C using the Brookhaven slow-chopper facility. Each spectrum exhibits two peaks that are characteristic of optical modes. The spectra of ammonium carbonate and ammonium citrate are similar to those of the body-centered-cubic lattice phase of the ammonium halides in which the ammonium ion has torsional and translational optical vibrations.

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