Resonantly enhanced optical nonlinearity in hybrid semiconductor quantum dot – metal nanoparticle structures

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The optical nonlinearity of hybrid structures composed of CdTe quantum dots and periodical particle array of gold is studied using Z-scan method. The optical nonlinearity is dramatically affected by the interaction between exciton in CdTe quantum dots and surface plasmons in Au periodical particle array. When the Au surface plasmon is tuned to be in resonance with the exciton transition in CdTe quantum dots, the largest nonlinear refractive index and the smallest two-photon absorption coefficient, n2 = −0.53 cm2/GW and β = 25 cm/GW, which are about 8 times larger and 50 times smaller than that of bare CdTe quantum dots, can be achieved.