Abstract

By using an effective independent-particle model for an interacting electron gas, the relaxation rate of excited electrons close enough to the Fermi surface is calculated. The theoretical description is based on a binary collision treatment, implemented by an approximate nonlinear characterization of the residual screened interactions and exact phase-shift calculations. The important constituents of a consistent attempt are discussed. The results obtained are analyzed and compared to those based on perturbative linear-screening predictions. Reductions in the lifetime of excited electrons are found. Comparisons with experimental data from different sources are made.

Highlights

  • One of the most important manifestations of electronelectron interaction in the conventional theory of a freeelectron gas is dielectric screening

  • ͓exp(Ϫt/␶)͔ that determine the decay of distributions for particles prepared in given momentum-energy states close to the invariant Fermi surface

  • An interpretation of this decay as a finite lifetime implies an uncertainty in the one-particle energy

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Summary

Introduction

One of the most important manifestations of electronelectron interaction in the conventional theory of a freeelectron gas is dielectric screening. The dielectric function itself is an exact mathematical property of the interacting system, but can only be calculated approximately. The random phase approximationRPAis a well-known example. It is, a generalized self-consistent procedure, which may be derived[1] by making the linearized Hartree equations time dependent in the treatment of the influence of a given external fieldthe field of a moving, charged particleon the system. For a heavy impurity one can apply density functional theoryDFT, which is a characteristic nonperturbative method of many-body theory.[4,5,6] For a light impurity one can use a self-consistent, Kahana-type[7] calculation, based on the Bethe-Goldstone formalism.[8]

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