Abstract

Semiconductor microcavities are often influenced by structural imperfections, which can disturb the flow and dynamics of exciton-polariton condensates. Additionally, in exciton-polariton condensates there is a variety of dynamical scenarios and instabilities, owing to the properties of the incoherent excitonic reservoir. We investigate the dynamics of an exciton-polariton condensate which emerges in semiconductor microcavity subject to disorder, which determines its spatial and temporal behaviour. Our experimental data revealed complex burst-like time evolution under non-resonant optical pulsed excitation. The temporal patterns of the condensate emission result from the intrinsic disorder and are driven by properties of the excitonic reservoir, which decay in time much slower with respect to the polariton condensate lifetime. This feature entails a relaxation oscillation in polariton condensate formation, resulting in ultrafast emission pulses of coherent polariton field. The experimental data can be well reproduced by numerical simulations, where the condensate is coupled to the excitonic reservoir described by a set of rate equations. Theory suggests the existence of slow reservoir temporarily emptied by stimulated scattering to the condensate, generating ultrashort pulses of the condensate emission.

Highlights

  • The formation process of an exciton polariton condensate[24, 25]

  • We study nontrivial dynamics of a polariton condensate created in a semiconductor microcavity with significant disorder[29]

  • This scenario holds in our case where one has to take into account the properties of incoherent reservoir relaxation[23] and long excitonic reservoir lifetime γR = 1/τR

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Summary

Introduction

The formation process of an exciton polariton condensate[24, 25]. In particular, nonequilibrium driven-dissipative condensates are much more influenced by disorder than their thermodynamic counterparts, where lack of the condensate stabilisation and superfluidity is predicted under any particle density[26,27,28]. We analyse near-field photoluminescence patterns to investigate the temporal dynamics of the system in a time-resolved experiment. It reveals complex oscillatory behaviour at long propagation distances and densities above the condensation threshold. The excitonic reservoir is temporarily burnt out by the condensate and needs to be replenished by relaxing high-energy electron-hole pairs to reach once again the condensation threshold density. These results can be reconstructed well by theoretical simulations within the phenomenological mean field approach taking into account a set of rate equations describing the exciton formation dynamics in the quantum well. Theoretical simulations suggest that the pulsating dynamics are the natural state of the condensate emission for a parameter set tuned to the properties of investigated sample

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