Abstract

Atmospheric new particle formation (NPF) events taking place over large distances between locations, featuring similar characteristics, have been the focus of studies during the last decade. The exact mechanism which triggers NPF still remains indefinable, so are the circumstances under which simultaneous occurrence of such events take place in different environments, let alone in environments which are parted by over 1200 km. In this study, concurrent number size distribution measurements were conducted in the urban environments of Athens (Greece) and Amman (Jordan) as well as the regional background site of Finokalia, Crete, all located within a distance of almost 1300 km for a 6-month period (February–July 2017). During the study period Athens and Finokalia had similar occurrence of NPF (around 20%), while the occurrence in Amman was double. When focusing on the dynamic characteristics at each site, it occurs that formation and growth rates at Amman are similar to those at Finokalia, while lower values in Athens can be ascribed to a higher pre-existing particle number at this urban site. By comparing common NPF events there are 5 concomitant days between all three sites, highly related to air masses origin. Additionally, for another 19 days NPF takes place simultaneously between Finokalia and Amman, which also share common meteorological characteristics, adding to a total of 60% out of 41 NPF events observed at Finokalia, also simultaneously occurring in Amman.

Highlights

  • IntroductionAtmospheric new particle formation (NPF) is a phenomenon involving the nucleation of gas-phase atmospheric components into newly-formed particles, as well as their subsequent growth and coagulation

  • Publisher’s Note: MDPI stays neutral with regard to jurisdictional claims in published maps and institutional affiliations.Atmospheric new particle formation (NPF) is a phenomenon involving the nucleation of gas-phase atmospheric components into newly-formed particles, as well as their subsequent growth and coagulation

  • It should be mentioned that Ntotal was considerably larger in Amman compared to Thissio by almost 85%, and this feature can be related to enhanced urban characteristics prevailing in Amman, since the Scanning Mobility Particle Sizers (SMPS) was situated close to overcrowded areas, and central roads

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Summary

Introduction

Atmospheric new particle formation (NPF) is a phenomenon involving the nucleation of gas-phase atmospheric components into newly-formed particles, as well as their subsequent growth and coagulation. Regional NPF events can be detected when a distinct burst of aerosol particles with diameters below 25 nm occurs, and the newly-formed mode is maintained for several hours [4]. Unlike regional events, during local-scale NPF events an intense appearance of a new mode in the particle number size distribution is observed, without subsequent growth; these events commonly exhibit strong intensity and limited duration [5]. It is deemed necessary to perform concurrent submicron particle number size distribution (PNSD) measurements at sites nearby, in order to assess the regional scale of NPF

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