Abstract

Graphene has been extensively investigated for its use in flexible electronics, especially graphene synthesized by chemical vapor deposition (CVD). To enhance the flexibility of CVD graphene, wrinkles are often introduced. However, reports on the flexibility of reduced graphene oxide (RGO) films are few, because of their weak conductivity and, in particular, poor flexibility. To improve the flexibility of RGO, reduced graphene oxide nanoshells are fabricated, which combine self-assembled polystyrene nanosphere arrays and high-temperature thermal annealing processes. The resulting RGO films with nanoshells present a better resistance stabilization after stretching and bending the devices than RGO without nanoshells. The sustainability and performance advances demonstrated here are promising for the adoption of flexible electronics in a wide variety of future applications.

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