Abstract
Self-powered photodetectors constructed by two-dimensional (2D) materials are significant in advanced science and technology with the growing focus on green and energy-efficient solutions. The built-in electric field in photodetector drives efficient separation and transfer of photogenerated electron–hole pairs. However, traditional metal-2D material-metal structures have more interface defects and larger Schottky barrier to hinder carrier transport. In this work, an asymmetric electrode material structure is constructed by adding graphene to provide a more efficient transport channel for photogenerated carriers. Graphene electrodes can play a variety of roles in efficient separation and collection of photogenerated carriers, reducing the barrier and improving the contact quality. Compared with the device using symmetric gold electrodes, the device prepared with asymmetric contacts show optimized performance. The MoTe2/WSe2 heterostructure exhibits brilliant self-powered photoresponse (a responsivity of 268 mA/W and a detectivity of 7.48*1011 Jones). And the rise/decay times are up to 145μs/125μs. Additionally, the detector has a broadband detection capability from visible light to near-infrared. These results provide a promising and simple way to fabricate a MoTe2/WSe2 self-powered broadband photodetector with high performance
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