Abstract
Reactions of trimethylaluminium, dimethylaluminium chloride and methylaluminium dichloride with methacrylonitrile have been investigated. These reactions afford corresponding donor-acceptor complexes. At elevated temperatures they react to yield methyl isopropenyl ketone (upon hydrolysis) and oligomers. During these reactions methane is formed in small amounts. The yield of reaction products has been studied in relation to the nature of methylaluminium compound and the reaction temperature.
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