Abstract
The reactions of trimethylaluminium, dimethylaluminium chloride, and methylaluminium dichloride with acrylonitrile have been investigated. They have been found to afford equimolecular donor-acceptor complexes. The complexes react at elevated temperatures to yield methane and derivatives of dihydro and hexahydro-pyrimidine. The yields of the products of the methylaluminium compounds investigated have been studied in relation to the reaction temperature. Reaction mechanisms have been discussed in terms of the data obtained.
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