Abstract

We describe the results of a five-month study during which 222Rn (radon) concentration, air- exchange (or ventilation) rate, and weather and radon source parameters were continuously monitored in a house near Chicago, with a view to accounting for the radon entry rate. The results suggest that the basement sump and perimeter drain-tile system played an important role in influencing the radon entry rate and that pressure-driven flow was more important than diffusion as a mechanism for radon entry. For the first 15 weeks of the study period the mean indoor radon concentration and air-exchange rate were 2.6 pCiℓ −1 (96 Bq m −3) and 0.22h −1, respectively; both parameters varied over a wide range. Radon concentration measured at the sump cover varied bimodally between 0 and 10 pCiℓ −1 (0–400 Bqm −3) and 300–700 pCiℓ −1 (10,000–30,000 Bq m −3). These two modes corresponded well to periods of low and high indoor radon concentration; average indoor concentrations for these periods were 1.5 and 6.5 pCiℓ −1 (55 and 240 Bq m −3), respectively. For data sorted into two groups according to radon activity at the sump, the indoor radon concentration showed little dependence on air-exchange rate. This result is accounted for by a model in which the radon entry rate, determined by mass balance, has two components—one diffusive, the other a pressure-driven flow component which is presumed to be proportional to the air-exchange rate. In fitting this model to the data we found that (1) the flow component dominated the diffusive component for periods of both high and low activity at the sump and (2) the magnitude of the diffusive component agreed well with the expected contributions of radon emanating from concrete and soil and diffusing into the house. To account for the flow component, we hypothesize that pressure drives air carrying a high concentration of radon generated in the soil, either through the bulk of the soil or along the outside of the basement walls, then into the basement through cracks and openings. During the final six weeks of the study, measurements were made with the water level in the sump maintained first below, then above the entrance of the pipe connected to the perimeter drain tile system. Average indoor radon concentrations during these two periods were 10.6 and 3.5 pCiℓ −1 (390 and 130 Bq m −3), respectively. The relatively high latter value compared with the mean for the first 15 weeks, combined with the observation of intervals of high airborne alpha activity at the sump during this period, suggest that the level of water in the sump does not, by itself, account for the variation in alpha activity at the sump that we had previously observed. Fireplace operation substantially increased the air-exchange rate, but had only a small effect on indoor radon concentration, providing corroborative evidence that pressure-driven flow is an important mechanism for radon entry into this house.

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