Abstract

Electronic and nuclear wavepackets created by coherent excitation of an autoionized and predissociated 'complex' resonance in H2 are studied theoretically using time-dependent multichannel quantum defect theory. The calculations predict that quantum beats between the components of the complex resonance interfere with Rydberg wavepacket (Kepler) motion to yield characteristic 'mixed' flux patterns in the observable time-dependent ionization and dissociation signals.

Full Text
Paper version not known

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call