Abstract

The dynamics of ionization waves (IWs) in atmospheric pressure discharges is fundamentally determined by the electric polarity (positive or negative) at which they are generated and by the presence of memory effects, i.e. leftover charges and reactive species that influence subsequent IWs. This work examines and compares positive and negative IWs in pulsed plasma jets (1 upmu s on-time), showing the difference in their nature and the different resulting interaction with a dielectric BSO target. For the first time, it is shown that a surface charging memory effect is produced, i.e. that a significant amount of surface charges and electric field remain in the target in between discharge pulses (200 upmu s off-time). This memory effect directly impacts IW dynamics and is especially important when using negative electric polarity. The results suggest that the remainder of surface charges is due to the lack of charged particles in the plasma near the target, which avoids a full neutralization of the target. This demonstration and the quantification of the memory effect are possible for the first time by using an unique approach, assessing the electric field inside a dielectric material through the combination of an advanced experimental technique called Mueller polarimetry and state-of-the-art numerical simulations.

Highlights

  • Plasma jets are very interesting for the study of interactions between low-temperature plasmas at atmospheric pressure and surfaces

  • ionization waves (IWs) propagate in a noble gas that flows through a dielectric tube and expands into air, forming a plume, where the discharge interacts with target surfaces

  • We have shown that combining electric field measurements in He plasma jets with plasma simulations provides a highly reliable and detailed characterization of electric field and surface charge on ­targets[34,35,36]

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Summary

Introduction

Plasma jets are very interesting for the study of interactions between low-temperature plasmas at atmospheric pressure and surfaces In these devices, IWs propagate in a noble gas that flows through a dielectric tube and expands into air, forming a plume, where the discharge interacts with target surfaces. In this article we show how the choice of applied voltage pulse affects the surface charging dynamics and the leftover charges and electric field in a BSO dielectric target impacted by a plasma jet. The differences of discharge dynamics and interaction with the dielectric BSO target for the different pulses of applied voltage are presented These reveal, for the first time, the direct influence of leftover surface charges as memory effect. This includes the description of how leftover surface charges are considered in simulations, why is pulse width slightly different in experiments and simulations and how to compare results in such conditions

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