Abstract

Functional plastic scintillators have attracted much attention for their usefulness in on-site monitoring and detection in environments. In this study, we elucidated a highly reliable and functional plastic scintillator for detection of radioactive strontium, which means a potent perovskite-loaded polymeric scintillation material based on epoxy and 2,5-diphenyloxazole (PPO). Moreover, Monte Carlo N-Particle (MCNP) simulation was performed to optimize the thickness of a plastic scintillator for efficient strontium detection. A thickness of 2 mm was found to be the optimum thickness for strontium beta-ray detection. A newly developed plastic scintillator with 430 nm emission from perovskite loading could trigger scintillation enhancement employing potential indication of perovskite energy transfer into a photomultiplier (PMT) detector. Furthermore, the response to beta-ray emitter of 90Sr was compared to commercial scintillator of BC-400 by exhibiting detection efficiency in the energy spectrum with a fabricated perovskite-loaded plastic scintillator. We believe that this suggested functional plastic scintillator could be employed as a radiation detector for strontium detection in a wide range of applications including decommissioning sites in nuclear facilities, nuclear security and monitoring, nonproliferation, and safeguards.

Highlights

  • Published: 8 March 2021In general, radioactive strontium as a fission product is one of the common radioisotopes found at the decommissioning sites in nuclear facilities

  • 10 g epoxy and 10 g hardener monomer were mixed in a bottle with PPO (0.2 wt%), POPOP (0.01 wt%), and perovskite (0.5 wt%) for characteristic evaluation and detection efficiency comparison to demonstrate the scintillation enhancement through the Förster Resonance Energy Transfer (FRET) mechanism occurring inside the scintillator

  • Plastic scintillator materials have been employed as radiation detectors in many areas including nuclear security, nonproliferation, safeguards, and basic science and technology

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Summary

Introduction

Published: 8 March 2021In general, radioactive strontium as a fission product is one of the common radioisotopes found at the decommissioning sites in nuclear facilities. 90 Sr is the most abundant radioisotope that remains in the 20~30 years later of the nuclear power plant’s decommissioning sites [1]. Radiation measurements such as dosimetry and dose controls are carried out by Geiger–Muller (GM) counter, gas proportional counter, or liquid scintillation counter (LSC) by measuring the high energy beta-ray emitted by 90 Y [1,2,3]. 90 Y from radioactive strontium is accumulated in the pancreas, which can lead to a number of problems in the body, such as cancer [6]

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