Polaron dynamics and decoherence in an interacting two-spin system coupled to an optical-phonon environment

Abstract

We study two anisotropically interacting spins coupled to optical phonons; we restrict our analysis to the regime of strong coupling to the environment, to the antiadiabatic region, and to the subspace with zero value for $S^z_T$ (the z-component of the total spin). In the case where each spin is coupled to a different phonon bath, we assume that the system and the environment are initially uncorrelated (and form a simply separable state) in the polaronic frame of reference. By analyzing the {polaron} dynamics through non-Markovian quantum master equation, we find that the system manifests a small amount of decoherence that decreases both with increasing non-adiabaticity and with enhancing strength of coupling; whereas, under the Markovian approximation, the polaronic system exhibits a decoherence free behavior. For the situation where both spins are coupled to the same phonon bath, we also show that the system is decoherence free in the subspace where $S^z_T$ is fixed. To suppress decoherence through quantum control, we employ a train of pi pulses and demonstrate that unitary evolution of the system can be retained. We propose realization of a weakly decohering charge qubit from an electron in an oxide-based (tunnel-coupled) double quantum dot system.