Abstract

Two-dimensional semiconductors inside optical microcavities have emerged as a versatile platform to explore new hybrid light–matter quantum states. A strong light–matter coupling leads to the formation of exciton-polaritons, which in turn interact with the surrounding electron gas to form quasiparticles called polaron-polaritons. Here, we develop a general microscopic framework to calculate the properties of these quasiparticles, such as their energy and the interactions between them. From this, we give microscopic expressions for the parameters entering a Landau theory for the polaron-polaritons, which offers a simple yet powerful way to describe such interacting light–matter many-body systems. As an example of the application of our framework, we then use the ladder approximation to explore the properties of the polaron-polaritons. Furthermore, we show that they can be measured in a non-demolition way via the light transmission/reflection spectrum of the system. Finally, we demonstrate that the Landau effective interaction mediated by electron-hole excitations is attractive leading to red shifts of the polaron-polaritons. Our work provides a systematic framework to study exciton-polaritons in electronically doped two-dimensional materials such as novel van der Waals heterostructures.

Highlights

  • Semiconductors in optical microcavities constitute a rich setting for exploring hybrid light–matter quantum systems with potential optoelectronic applications [1,2]

  • Photons in the cavity are strongly coupled to excitons in the semiconductor and the excitons in turn interact with a 2D electron gas (2DEG)

  • We presented a theoretical framework for describing polaron-polaritons in 2D semiconductors inside optical microcavities

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Summary

Introduction

Semiconductors in optical microcavities constitute a rich setting for exploring hybrid light–matter quantum systems with potential optoelectronic applications [1,2]. The large binding energy of excitons in TMDs as compared to other microcavity semiconductors such as quantum-wells [32,33,34], combined with the possibility to control the electron density in the different valleys, opens up exciting new venues to explore Bose–Fermi mixtures in a hybrid light–matter setting [35,36,37] This has stimulated a number of studies regarding the properties electron–exciton mixtures and their coupling to light [38,39,40,41,42,43,44,45,46,47,48].

System
Fermi Polaron-Polaritons
Microscopic Theory
Landau Theory
The Ladder Approximation
Zero Polaron-Polariton Density
Non-Zero Polaron-Polariton Density
Conclusions
Full Text
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