Plasmonic Bound States in the Continuum to Tailor Exciton Emission of MoTe2.

Abstract

Plasmon resonances can greatly enhance light-matter interactions of two-dimensional van der Waals materials. However, the quality factor of plasmonic resonances is limited. Here, we demonstrate a plasmonic quasi-bound state in the continuum (quasi-BIC), which is composed of gold nanorod pairs. Through controlling the rotation angle of the nanorods, the quality factor of the plasmonic BIC mode can be tuned. Simulation results show that the plasmonic BIC combines the advantages of high-quality factor from the BIC effect and small mode volume from plasmonic resonance. Experiment results show that the designed plasmonic BIC mode exhibits a quality factor higher than 15 at the wavelength of around 1250 nm. Through integrating the plasmonic bound state structure with monolayer molybdenum ditelluride (MoTe2), the exciton emission of MoTe2 in the PL spectrum split into two exciton-polariton modes, which is attributed to the high Q factor and strong interaction between the BIC mode and excitons of MoTe2.