Photothermal-driven flow with water droplets for effective removal of indoor fine particulate matters

Abstract

Airborne particulate matter (PM) causes hazardous problems in human health, and water droplets have been utilized for PM removal in the air. However, since conventional wet scrubbing techniques mostly rely on mechanically generated water droplets, they have intrinsically limited in collection efficiencies of a single droplet. In addition, PM capturing strategies for removal of fine PM need to be established to enhance PM removal performance based on flow dynamics. Here, we propose a steam flow of water droplets generated by a photothermal membrane for air purification. The generated flow captures PM efficiently by the aid of the coupled effects of water droplets and hydrodynamic flow. The flow achieves high and sustainable deposition constants of 0.458 and 0.472 h−1 for PM1.0 and PM2.5 within 1 h at 4 solar intensity, which is 2.20 and 2.24 times higher than those of without solar irradiation, respectively. The deposition constants of PM using steam flow were higher than that of previous wet scrubbing methods despite a low volume of water usage. Our photothermal-driven flow with water droplets could be utilized as effective indoor air purification system that is low cost, energy-efficient, and environmentally-friendly.