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Abstract
Irradiation of a mixture of 1,3-dienes, silanes, and pentacarbonyliron leads to mixtures of isomeric hydrosilylation products. The reaction is shown to proceed via the intermediate formation of (η 3- anti-butenyl)tricarbonyliron-trialkylsilicon complexes which are accessible by photoinduced addition of R 3SiH to (η 4-butadiene)tricarbonyliron and, upon thermal decomposition, yield similar mixtures of isomeric butenyltrialkyisilicon derivatives.
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