Abstract

Abstract We report new organic-inorganic hybrid gate insulator materials containing solution-processable zinc diacrylate (ZnDA) and dipentaerythritol penta-/hexa-acrylate (DPHA) to fabricate high-performance and reliable organic thin film transistors (OTFTs). ZnDA-DPHA organic-inorganic hybrid materials can be crosslinked by ultraviolet illumination (λmax = 365 nm) within 7 min in the presence of a photoinitiator. Hence, the crosslinked insulator film provides not only good insulating properties (such as a dielectric constant of ca. 4.95 and low leakage current of

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